第4期 曹芳等:碳质气溶胶的放射性碳同位素(“C)源解析:原理、方法和研究进展 431 ods in Physics Research Section B-Beam Interactions with Materi- [37 Yang F, He K, Ye B, et al. One-year record of organic and ele- als and Atoms,2010,268(17/18):2831-2834. mental carbon in fine particles in downtown Beijing and Shanghai [24 Szidat S, Ruff M, Perron N, et al. Fossil and non-fossil sources [J. Atmospheric Chemistry and Physics, 2005, 5: 1 449-1 457 of Organic Carbon(OC)and Elemental Carbon(EC)in Goete- [38] Liu D, Li J, Zhang Y, et al. The use of levoglucosan and radio- borg[ J]. Sweden Atmospheric Chemistry and Physics, 2009,9 carbon for source apportionment of PM, s carbonaceous aerosols at 1521-1535 a background site in East China[J]. Environmental Science and [25] Zhang Y L, Perron N, Ciobanu V G, et al. On the isolation of hnology,2013,47(18):10454-10461 OC and EC and the optimal strategy of radiocarbon-based source [39] Liu J, Li J, Zhang Y, et al. 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Summary of organic and elemental car鄄 bon / black carbon analysis methods and intercomparisons [ J]. Aerosol and Air Quality Research, 2005, 5(1): 65鄄102. [33] Yang H, Yu J Z. Uncertainties in charring correction in the anal鄄 ysis of elemental and organic carbon in atmospheric particles by thermal / optical methods[J]. Environmental Science and Technol鄄 ogy, 2002, 36(23): 5 199鄄5 204. [34] Zhang Y L, Perron N, Ciobanu V G, et al. On the isolation of OC and EC and the optimal strategy of radiocarbon—based source apportionment of carbonaceous aerosols[J]. Atmospheric Chemis鄄 try and Physics Discussions, 2012, 12: 17 657鄄17 702. [35] Yu J Z, Xu J, Yang H. Charring characteristics of atmospheric organic particulate matter in thermal analysis[ J]. Environmental Science and Technology, 2002, 36(4): 754鄄761. [36] Shao Min, Li Jinlong, Tang Xiaoyan. Source apportionment of atmospheric carbonaceous aerosols using AMS [ J]. Journal of Nuclear and Radiochemistry, 1996, 18 (4): 234鄄238. [ 邵敏, 李金龙, 唐孝炎. 大气气溶胶含碳组分的来源研究———加速 器质谱法[J]. 核化学与放射化学, 1996, 18(4): 234鄄238. ] [37] Yang F, He K, Ye B, et al. One鄄year record of organic and ele鄄 mental carbon in fine particles in downtown Beijing and Shanghai [ J]. Atmospheric Chemistry and Physics, 2005, 5: 1 449鄄1 457. [38] Liu D, Li J, Zhang Y, et al. The use of levoglucosan and radio鄄 carbon for source apportionment of PM2. 5 carbonaceous aerosols at a background site in East China[ J]. Environmental Science and Technology, 2013, 47(18): 10 454鄄10 461. [39] Liu J, Li J, Zhang Y, et al. Source apportionment using radio鄄 carbon and organic tracers for PM2. 5 carbonaceous aerosols in Guangzhou, South China: Contrasting local鄄and regional鄄scale haze events[ J]. Environmental Science and Technology, 2014, 48(20):12 002鄄12 011. [40] Song J, He L, Peng P A, et al. Chemical and isotopic compos鄄 tion of Humic鄄Like Substances ( HULIS) in ambient aerosols in Guangzhou, South China [ J]. Aerosol Science and Technology, 2012, 46(5): 533鄄546. [41] Zhang Y, Liu J, Salazar G A, et al. Micro鄄scale (滋g) radiocar鄄 bon analysis of water鄄soluble organic carbon in aerosol samples [J]. Atmospheric Environment, 2014, 97: 1鄄5. [42] Szidat S, Bench G, Bernardoni V, et al. Intercomparison of 14C analysis of carbonaceous aerosols: Exercise 2009[ J]. Radiocar鄄 bon, 2013, 55(3 / 4): 1 496鄄1 509. [43] Reddy C M, Pearson A, Xu L, et al. Radiocarbon as a tool to apportion the sources of polycyclic aromatic hydrocarbons and black carbon in environmental samples[ J]. Environmental Sci鄄 ence and Technology, 2002, 36(8): 1 774鄄1 782. [44] Mollenhauer G, Rethemeyer J. Compound鄄specific radiocarbon a鄄 nalysis鄄Analytical challenges and applications[C]椅IOP Confer鄄 ence Series: Earth and Environmental Science Program 5, 2009. [45] Mandalakis M, Gustafsson O, Alsberg T, et al. Contribution of biomass burning to atmospheric polycyclic aromatic hydrocarbons at three European background sites [ J]. Environmental Science and Technology, 2005, 39(9):2 976鄄2 982. [46] Fahrni S M, Ruff M, Wacker L, et al. A preparative 2D鄄chro鄄 matography method for compound鄄specific radiocarbon analysis of dicarboxylic acids in aerosols[ J]. Radiocarbon, 2010, 52(2): 752鄄760. [47] Wacker L, Fahrni S M, Hajdas I, et al. A versatile gas interface for routine radiocarbon analysis with a gas ion source[J]. Nucle鄄 ar Instruments and Methods in Physics Research Section B—Beam Interactions with Materials and Atoms, 2013, 294: 315鄄319. [48] Wacker L, Bonani G, Friedrich M, et al. Micadas: Routine and high鄄precision radiocarbon dating [ J]. Radiocarbon, 2010, 52 (2): 252鄄262. [49] Uhl T, Luppold W, Rottenbach A, et al. Development of an au鄄 tomatic gas handling system for microscale AMS 14C measure鄄 ments[J]. Nuclear Instruments and Methods in Physics Research Section B—Beam Interactions with Materials and Atoms, 2007, 259: 303鄄307. [50] Szidat S, Salazar G A, Vogel E, et al. 14C analysis and sample preparation at the new bern Laboratory for the Analysis of Radio鄄 carbon with AMS ( LARA) [ J]. Radiocarbon,2014, 56 ( 2 ): 第 4 期 曹 芳等:碳质气溶胶的放射性碳同位素( 431 14C)源解析:原理、方法和研究进展