71 环境化学 33卷 Eastern China [n. Atmos Environ, 2008, 42(25): 6321-6334 [55] Bundke U, Hanel G, Horvath H, et al. Aerosol optical properties during the Lindenberg Aerosol Characterization Experiment (LACE 98) D. J Geophys Res-Atmos, 2002, 107(D21) 6] Eldering A, Ogren J A, Chowdhury Z, et al. Aerosol optical properties during INDOEX based on measured aerosol particle size and composition [I. J Geophys Res-Atmos, 2002, 107(D22 57]杨军,李子华,黄世鸿、相对湿度对大气气溶胶粒子短波辐射特性的影响D].大气科学,199,23(2):239-47 [58] Jacobson M Z. Strong radiative heating due to the mixing state of black carbon in atmospheric aerosols []. Nature, 2001, 409(6821) 95-697 s9王雷,葛茂发,王炜罡.烟炱气溶胶的光学辐射特性研究D.环境化学,2011,30(1):120-129 [60] Lesins G, Chylek P, Lohmann U. A study of intemal and extemal mixing scenarios and its effect on aerosol optical properties and direct radiative forcing [. J Geophys Res-Atmos, 2002, 107(D10) [61] Yang M, Howell S, Zhuang J, et al. Attribution of aerosol light absorption to black carbon, brown carbon, and dust in China- interpretations of atmospheric measurements during EAST-AIRE D]. Atmos Chem Phys, 2009,9(6): 2035-2050 [62] Moffet R C, Prather K A. Insitu measurements of the mixing state and optical properties of soot with implications for radiative forcing estimates D]. Proceedings of the National Academy of Sciences, 2009, 106(29): 11872-11877 [63] Schnaiter M, Linke C, Mohler 0, et al. Absorption amplification of black carbon intemally mixed with secondary organic aerosol DI Journal of Geophysical Research: Atmospheres (1984--2012), 2005,110(D19) [64] Adachi K, Buseck P. Internally mixed soot, sulfates, and organic matter in aerosol particles from Mexico City [I. Atmos Chem Phys 2008,8(21):6469-6481 [65] Horvath H. Atmospheric light absorptior-A review [I. Atmos Environ Part A General Topics, 1993,27(3): 293-317 [66] Fuller K A, Malm W C, Kreidenweis S M. Effects of mixing on extinction by carbonaceous particles []. Journal of Geophysical Research: Atmospheres(1984-2012),1999,104(D13):15941-15954 [67] Heintzenberg J. Light scattering parameters of internal and extemal mixtures of soot and non absorbing material in atmospheric aerosols [C]. Proceedings of the Conference on Carbonaceous Particles in the Atmosphere: 1978 8] Bond T C, Habib G, Bergstrom RW. Limitations in the enhancement of visible light absorption due to mixing state [].Journal of Geophysical Research: Atmospheres(1984--2012), 2006, 111(D20) ⑨]郝丽,杨文,吴统文,等.黑碳-酸盐混合气溶胶的辐射特性分析⑩.高原气象,2010,29(5):1238-1245 [70] Cheng Y F, Eichler H, Wiedensohler A, et al. Mixing state of elemental carbon and non-ight-absorbing aerosol components derived from in situ particle optical properties at Xinken in Pearl River Delta of China [n. Joumal of Geophysical Research: Atmospheres(1984- 2012),2006,111(D20) 1] Khalizov A F, Xue H, Wang L, et al. Enhaneed light absorption and scattering by carbon soot aerosol intemally mixed with sulfuric acid D. The Journal of Physical Chemistry A, 2009, 113(6):1066-1074 72] Zhang R, Khalizoy A F, Pagels J, et al. Variability in morphology, hygroscopicity, and optical properties of soot aerosols during mospheric processing [I. Proceedings of the National Academy of Sciences, 2008, 105(30): 10291-10296 [73] Yu H, Wu C, Wu D,et al. Size distributions of elemental carbon and its contribution to light extinction in urban and rural locations in the pearl river delta region, China [. Atmos Chem Phys, 2010,10(11): 5107-5119 [74] Mallet M, Roger J, Despiau S, et al. A study of the mixing state of black carbon in urban zone []. Joumal of Geophysical Research: morphemes(1984-2012),2004,109(D4) [75]Covert D S, Heintzenberg J. Measurement of the degree of internal /external mixing of hygroscopic compounds and soot in atmospheric aerosols [ Sci Total Environ, 1984, 36: 347-352 [76] Charlson R, Anderson T, Rodhe H. Direct climate forcing by anthropogenic aerosols: Quantifying the link between atmospheric sulfate and diation [n. Contributions to atmospheric physics, 1999,72(1): 79-94 [77] Yuan C S, Lee C G, Liu S H, et al. Correlation of atmospheric visibility with chemical composition of Kaohsiung aerosols [.Atmos Res,2006,82(3):663-679 [78] Hand J, Copeland D, Day A, et al. Spatial and seasonal patterns and temporal variability of haze and its constituents in the United States: Report V: June 2011 [R]. Cooperative Institute for Research in the Atmosphere for the IMPROVE program, 2011 9] Malm W C, Hand J L. An examination of the physical and optical properties of aerosols collected in the IMPROVE program [.Atmos environ,2007,41(16):3407-427 8o]姚婷婷,黄晓锋,何凌燕,等.深圳市冬季大气消光性质与细粒子化学组成的高时间分辨率观测和统计关系研究口.中国科 学:化学,2010(8):1163-171 [81] McDonald K, Shepherd M. Characterization of visibility impacts related to fine particulate matter in Canada []. J Air Waste Manage 2004,54(9):1061-1068 [82] Yang LX, Wang D C, Cheng S H, et al. Influence of meteorological conditions and particulate matter on visual range impairment in Jinan China [] Sci Total Environ, 2007, 383(1):164-173 21994-2014ChinaAcademicJOurnalElectronicpUblishingHouse.Allrightsreservedhttp:/www.cnki.net714 环 境 化 学 33 卷 Eastern China ［J］． Atmos Environ，2008，42( 25) : 6321-6334 ［55］ Bundke U，Hanel G，Horvath H，et al． Aerosol optical properties during the Lindenberg Aerosol Characterization Experiment ( LACE 98) ［J］． J Geophys Ｒes-Atmos，2002，107( D21) ［56］ Eldering A，Ogren J A，Chowdhury Z，et al． Aerosol optical properties during INDOEX based on measured aerosol particle size and composition ［J］． J Geophys Ｒes-Atmos，2002，107( D22) ［57］ 杨军，李子华，黄世鸿． 相对湿度对大气气溶胶粒子短波辐射特性的影响 ［J］． 大气科学，1999，23( 2) : 239-247 ［58］ Jacobson M Z． Strong radiative heating due to the mixing state of black carbon in atmospheric aerosols ［J］． Nature，2001，409( 6821) : 695-697 ［59］ 王雷，葛茂发，王炜罡． 烟炱气溶胶的光学辐射特性研究 ［J］． 环境化学，2011，30( 1) : 120-129 ［60］ Lesins G，Chylek P，Lohmann U． A study of internal and external mixing scenarios and its effect on aerosol optical properties and direct radiative forcing ［J］． J Geophys Ｒes-Atmos，2002，107( D10) ［61］ Yang M，Howell S，Zhuang J，et al． Attribution of aerosol light absorption to black carbon，brown carbon，and dust in China￾interpretations of atmospheric measurements during EAST-AIＲE ［J］． Atmos Chem Phys，2009，9( 6) : 2035-2050 ［62］ Moffet Ｒ C，Prather K A． In-situ measurements of the mixing state and optical properties of soot with implications for radiative forcing estimates［J］． Proceedings of the National Academy of Sciences，2009，106( 29) : 11872-11877 ［63］ Schnaiter M，Linke C，Mhler O，et al． Absorption amplification of black carbon internally mixed with secondary organic aerosol ［J］． Journal of Geophysical Ｒesearch: Atmospheres ( 1984—2012) ，2005，110( D19) ［64］ Adachi K，Buseck P． Internally mixed soot，sulfates，and organic matter in aerosol particles from Mexico City ［J］． Atmos Chem Phys， 2008，8( 21) : 6469-6481 ［65］ Horvath H． Atmospheric light absorption—A review ［J］． Atmos Environ Part A General Topics，1993，27( 3) : 293-317 ［66］ Fuller K A，Malm W C，Kreidenweis S M． Effects of mixing on extinction by carbonaceous particles ［J］． Journal of Geophysical Ｒesearch: Atmospheres ( 1984—2012) ，1999，104( D13) : 15941-15954 ［67］ Heintzenberg J． Light scattering parameters of internal and external mixtures of soot and non-absorbing material in atmospheric aerosols ［C］． Proceedings of the Conference on Carbonaceous Particles in the Atmosphere; 1978 ［68］ Bond T C，Habib G，Bergstrom ＲW． Limitations in the enhancement of visible light absorption due to mixing state ［J］． Journal of Geophysical Ｒesearch: Atmospheres ( 1984—2012) ，2006，111( D20) ［69］ 郝丽，杨文，吴统文，等． 黑碳-硫酸盐混合气溶胶的辐射特性分析 ［J］． 高原气象，2010，29( 5) : 1238-1245 ［70］ Cheng Y F，Eichler H，Wiedensohler A，et al． Mixing state of elemental carbon and non-light-absorbing aerosol components derived from in situ particle optical properties at Xinken in Pearl Ｒiver Delta of China ［J］． Journal of Geophysical Ｒesearch: Atmospheres ( 1984— 2012) ，2006，111( D20) ［71］ Khalizov A F，Xue H，Wang L，et al． Enhanced light absorption and scattering by carbon soot aerosol internally mixed with sulfuric acid ［J］． The Journal of Physical Chemistry A，2009，113( 6) : 1066-1074 ［72］ Zhang Ｒ，Khalizov A F，Pagels J，et al． Variability in morphology，hygroscopicity，and optical properties of soot aerosols during atmospheric processing ［J］． Proceedings of the National Academy of Sciences，2008，105( 30) : 10291-10296 ［73］ Yu H，Wu C，Wu D，et al． Size distributions of elemental carbon and its contribution to light extinction in urban and rural locations in the pearl river delta region，China ［J］． Atmos Chem Phys，2010，10( 11) : 5107-5119 ［74］ Mallet M，Ｒoger J，Despiau S，et al． A study of the mixing state of black carbon in urban zone ［J］． Journal of Geophysical Ｒesearch: Atmospheres ( 1984—2012) ，2004，109( D4) ［75］ Covert D S，Heintzenberg J． Measurement of the degree of internal /external mixing of hygroscopic compounds and soot in atmospheric aerosols［J］． Sci Total Environ，1984，36: 347-352 ［76］ Charlson Ｒ，Anderson T，Ｒodhe H． Direct climate forcing by anthropogenic aerosols: Quantifying the link between atmospheric sulfate and radiation ［J］． Contributions to atmospheric physics，1999，72( 1) : 79-94 ［77］ Yuan C S，Lee C G，Liu S H，et al． Correlation of atmospheric visibility with chemical composition of Kaohsiung aerosols ［J］． Atmos Ｒes，2006，82( 3) : 663-679 ［78］ Hand J，Copeland D，Day A，et al． Spatial and seasonal patterns and temporal variability of haze and its constituents in the United States: Ｒeport V: June 2011［Ｒ］． Cooperative Institute for Ｒesearch in the Atmosphere for the IMPＲOVE program，2011 ［79］ Malm W C，Hand J L． An examination of the physical and optical properties of aerosols collected in the IMPＲOVE program ［J］． Atmos Environ，2007，41( 16) : 3407-3427 ［80］ 姚婷婷，黄晓锋，何凌燕，等． 深圳市冬季大气消光性质与细粒子化学组成的高时间分辨率观测和统计关系研究 ［J］． 中国科 学: 化学，2010( 8) : 1163-1171 ［81］ McDonald K，Shepherd M． Characterization of visibility impacts related to fine particulate matter in Canada ［J］． J Air Waste Manage， 2004，54( 9) : 1061-1068 ［82］ Yang L X，Wang D C，Cheng S H，et al． Influence of meteorological conditions and particulate matter on visual range impairment in Jinan， China ［J］． Sci Total Environ，2007，383( 1) : 164-173